Litcius/Paper detail

Atomic layer deposited Al <sub>2</sub> O <sub>3</sub> passivation layer for few-layer WS <sub>2</sub> field effect transistors

Young Gyu You, Dong Ho Shin, Jong Hwa Ryu, E. E. B. Campbell, Hyun‐Jong Chung, Sung Ho Jhang

2021Nanotechnology16 citationsDOIOpen Access PDF

Abstract

Abstract We have investigated the effect of an Al 2 O 3 passivation layer on the performance of few-layer WS 2 FETs. While the performance of WS 2 FETs is often limited by a substantial decrease in carrier mobility owing to charged impurities and a Schottky barrier between the WS 2 and metal electrodes, the introduction of an Al 2 O 3 overlayer by atomic layer deposition (ALD) suppressed the influence of charged impurities by high- κ dielectric screening effect and reduced the effective Schottky barrier height. We argue that n-doping of WS 2 , induced by positive fixed charges formed at Al 2 O 3 /WS 2 interface during the ALD process, is responsible for the reduction of the effective Schottky barrier height in the devices. In addition, the Al 2 O 3 passivation layer protected the device from oxidation, and maintained stable electrical performance of the WS 2 FETs over 57 d. Thus, the ALD of Al 2 O 3 overlayer provides a facile method to enhance the performance of WS 2 FETs and to ensure ambient stability.

Topics & Concepts

Materials sciencePassivationAtomic layer depositionSchottky barrierLayer (electronics)ImpurityDopingDielectricOptoelectronicsBarrier layerSchottky diodeField-effect transistorElectrodeAnalytical Chemistry (journal)TransistorNanotechnologyElectrical engineeringVoltagePhysical chemistryChromatographyDiodeOrganic chemistryChemistryEngineering2D Materials and ApplicationsMXene and MAX Phase MaterialsFerroelectric and Negative Capacitance Devices