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Meerwein‐type Bromoarylation with Arylthianthrenium Salts

Yuan Cai, Tobias Ritter

2022Angewandte Chemie International Edition70 citationsDOIOpen Access PDF

Abstract

Herein, we report a photocatalyzed Meerwein-type bromoarylation of alkenes with stable arylthianthrenium salts, formed by site-selective C-H thianthrenation. This protocol can be applied to late-stage functionalization of a variety of biomolecules that are difficult to access by other aryl coupling reagents. Halogen introduction allows for a variety of follow-up transformations, affording numerous biologically active skeletons.

Topics & Concepts

ReagentChemistryCombinatorial chemistryHalogenBiomoleculeArylSurface modificationOrganic chemistryBiochemistryAlkylPhysical chemistryCatalytic C–H Functionalization MethodsRadical Photochemical ReactionsOxidative Organic Chemistry Reactions
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