Litcius/Paper detail

1D Magneto-Optical Trap of Polyatomic Molecules

Louis Baum, Nathaniel B. Vilas, Christian Hallas, Benjamin L. Augenbraun, Shivam Raval, Debayan Mitra, John M. Doyle

2020Physical Review Letters101 citationsDOIOpen Access PDF

Abstract

We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasiclosed cycling transition is established to scatter ∼10^{3} photons per molecule, predominantly limited by interaction time. This enables radiative laser cooling of CaOH while compressing the molecular beam, leading to a significant increase in on axis beam brightness and reduction in temperature from 8.4 to 1.4 mK.

Topics & Concepts

Magneto-optical trapAtomic physicsPolyatomic ionLaserLaser coolingMoleculeTrap (plumbing)PhotonBeam (structure)MagnetoPhysicsBrightnessMolecular beamMaterials scienceRadiative transferOpticsIgnition systemQuantum mechanicsThermodynamicsMeteorologyCold Atom Physics and Bose-Einstein CondensatesQuantum Information and CryptographyStrong Light-Matter Interactions