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High Harmonic Generation in a Correlated Electron System

Shohei Imai, Atsushi Ono, Sumio Ishihara

2020Physical Review Letters81 citationsDOIOpen Access PDF

Abstract

High harmonic generation in crystalline solids has been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show the emergence of high harmonic generation signals which are attributed to the dynamics of many-body states in a low-dimensional correlated electron system. An interacting fermion model and its effective pseudospin model on a one-dimensional dimer-type lattice are analyzed. Observed high harmonic generation signals in a spontaneously symmetry-broken state, where charge densities are polarized inside of dimer units, show threshold behavior with respect to light amplitude and are interpreted in terms of tunneling and recombination of kink-antikink excitations in an electric field.

Topics & Concepts

PhysicsElectronQuantum tunnellingCondensed matter physicsHigh harmonic generationFermionLattice (music)AmplitudeElectric fieldAtomic physicsQuantum mechanicsAcousticsLaserLaser-Matter Interactions and ApplicationsSpectroscopy and Quantum Chemical StudiesAdvanced Chemical Physics Studies