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Validation of OMPS Suomi NPP and OMPS NOAA‐20 Formaldehyde Total Columns With NDACC FTIR Observations

Hyeong‐Ahn Kwon, Gonzalo González Abad, Caroline R. Nowlan, Heesung Chong, Amir H. Souri, Corinne Vigouroux, Amelie N. Röhling, Rigel Kivi, Maria Makarova, Justus Notholt, Mathias Palm, Holger Winkler, Yao Té, Ralf Sussmann, Markus Rettinger, Emmanuel Mahieu, Kimberly Strong, Erik Lutsch, Shoma Yamanouchi, Tomoo Nagahama, James W. Hannigan, Minqiang Zhou, Isao Murata, Michel Grutter, Wolfgang Stremme, Martine De Mazière, Nicholas Jones, Dan Smale, Isamu Morino

2023Earth and Space Science25 citationsDOIOpen Access PDF

Abstract

Abstract We validate formaldehyde (HCHO) vertical column densities (VCDs) from Ozone Mapping and Profiler Suite Nadir Mapper (OMPS‐NM) instruments onboard the Suomi National Polar‐orbiting Partnership (Suomi NPP) satellite for 2012–2020 and National Oceanic and Atmospheric Administration‐20 (NOAA‐20) satellite for 2018–2020, hereafter referred to as OMPS‐NPP and OMPS‐N20, with ground‐based Fourier‐Transform Infrared (FTIR) observations of the Network for the Detection of Atmospheric Composition Change (NDACC). OMPS‐NPP/N20 HCHO products reproduce seasonal variability at 24 FTIR sites. Monthly variability of OMPS‐NPP/N20 has a very good agreement with FTIR, showing correlation coefficients of 0.83 and 0.88, respectively. OMPS‐NPP (N20) biases averaged over all sites are −0.9 (4) ± 3 (6)%. However, at clean sites (with VCDs < 4.0 × 10 15 molecules cm −2 ), positive biases of 20 (32) ± 6 (18)% occur for OMPS‐NPP (N20). At sites with HCHO VCDs > 4.0 × 10 15 molecules cm −2 , negative biases of −15% ± 4% appear for OMPS‐NPP, but OMPS‐N20 shows smaller bias of 0.5% ± 6% due to its smaller ground pixel footprints. Therefore, smaller satellite footprint sizes are important in distinguishing small‐scale plumes. In addition, we discuss a bias correction and provide lower limit for the monthly uncertainty of OMPS‐NPP/N20 HCHO products. The total uncertainty for OMPS‐NPP (N20) at clean sites is 0.7 (0.8) × 10 15 molecules cm −2 , corresponding to a relative uncertainty of 32 (30)%. In the case of HCHO VCDs > 4.0 × 10 15 molecules cm −2 , however, the relative uncertainty in HCHO VCDs for OMPS‐NPP (N20) decreases to 31 (18)%.

Topics & Concepts

Environmental scienceSatelliteAtmospheric sciencesFormaldehydeFourier transform infrared spectroscopyRemote sensingMeteorologyChemistryPhysicsGeologyOpticsAstronomyOrganic chemistryAtmospheric Ozone and ClimateAtmospheric and Environmental Gas DynamicsAtmospheric chemistry and aerosols