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Bulk modulus of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi mathvariant="normal">H</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mi mathvariant="normal">O</mml:mi></mml:mrow></mml:math> across the ice VII–ice X transition measured by time-resolved x-ray diffraction in dynamic diamond anvil cell experiments

Alba San José Méndez, Florian Trybel, Rachel J. Husband, Gerd Steinle‐Neumann, Hanns‐Peter Liermann, Hauke Marquardt

2021Physical review. B./Physical review. B40 citationsDOI

Abstract

We have studied the ${\mathrm{H}}_{2}\mathrm{O}$ ice VII--ice X phase transition at room temperature by performing three quasicontinuous synchrotron time-resolved x-ray-diffraction experiments in a dynamic diamond anvil cell, reaching pressures of 180 GPa. The dense pressure coverage of our volume data allows us to directly derive the bulk modulus for ${\mathrm{H}}_{2}\mathrm{O}$ over the entire pressure range. Our data document three major changes in compression behavior in the ranges of 35--40, 50--55, and 90--110 GPa, likely corresponding to the formation of pretransition dynamically disordered ice VII and ice X, and static ice X, respectively. Our results confirm that ice X has a very high bulk modulus.

Topics & Concepts

Bulk modulusDiamond anvil cellMaterials scienceCrystallographyPhase transitionVolume (thermodynamics)PhysicsPhase (matter)Analytical Chemistry (journal)ThermodynamicsHigh pressureChemistryChromatographyQuantum mechanicsHigh-pressure geophysics and materialsMachine Learning in Materials ScienceChemical Thermodynamics and Molecular Structure
Bulk modulus of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi mathvariant="normal">H</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mi mathvariant="normal">O</mml:mi></mml:mrow></mml:math> across the ice VII–ice X transition measured by time-resolved x-ray diffraction in dynamic diamond anvil cell experiments | Litcius