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Mitochondrial-Targeted Ratiometric Fluorescent Probe to Monitor ClO− Induced by Ferroptosis in Living Cells

Beidou Feng, Kui Wang, Zhe Wang, Huiyu Niu, Ge Wang, Yuehua Chen, Hua Zhang

2022Frontiers in Chemistry12 citationsDOIOpen Access PDF

Abstract

Ferroptosis is a type of iron-dependent programmed cell death. Once such kind of death occurs, an individual cell would undergo a series of changes related to reactive oxygen species (ROS) in mitochondria. A mitochondrial-targeted ratiometric fluorescent probe ( MBI-OMe ) was developed to specifically detect ferroptosis-induced ClO − , whose recognition group is p -methoxyphenol, and the mitochondrial-targeted group is benzimidazole. The fluorescence of MBI-OMe was first quenched by 30 μM of Fe 3+ , and then MBI-OMe appeared as a ratiometric signal at 477 nm and 392 nm in response to ferroptosis-induced ClO − in living cells. MBI-OMe was successfully used to evaluate changes in ClO − induced by ferroptosis.

Topics & Concepts

FluorescenceProgrammed cell deathReactive oxygen speciesMitochondrionChemistryBenzimidazoleCellBiophysicsApoptosisOxygenPhotochemistryCell biologyBiochemistryBiologyPhysicsOrganic chemistryQuantum mechanicsDrug Transport and Resistance MechanismsTrace Elements in HealthAdvanced biosensing and bioanalysis techniques
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