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Na<sub>2</sub>O-Gd<sub>2</sub>O<sub>3</sub>-Al<sub>2</sub>O<sub>3</sub>-P<sub>2</sub>O<sub>5</sub> glass scintillator doped with Dy<sup>3+</sup>: X-rays and proton responses

N. Wantana, E. Kaewnuam, Y. Tariwong, Nguyen Duy Quang, P. Pakawanit, C. Phoovasawat, Naratip Vittayakorn, S. Kothan, H. J. Kim, J. Kaewkhao

2022Japanese Journal of Applied Physics27 citationsDOIOpen Access PDF

Abstract

Abstract Dy 3+ :Na 2 O-Al 2 O 3 -Gd 2 O 3 -P 2 O 5 (Dy:NAGP) glasses were fabricated to investigate the capability for radiation responses. The influence of Dy 2 O 3 concentration on glass properties was studied. The density and effective atomic number of glass increased with the addition of Dy 2 O 3 content. The glasses absorbed the photons in the ultraviolet, visible light, and near-infrared region. In photoluminescence (PL) spectra, the obvious yellow emission at 574 nm and blue emission at 482 nm of Dy 3+ were both generated by the direct excitation and the Gd–Dy energy transfer. The PL decay time of glasses was in the millisecond order. There was thermal quenching observed in temperature-dependent luminescence (TDL). The radioluminescence (RL) and protonluminescence (PrL) represented the emission pattern of Dy 3+ similarly to PL spectra. The concentration quenching caused 0.50Dy:NAGP glass with the highest PL and RL emission intensity. The X-ray imaging of developed glass using a synchrotron light source was successfully imaged for the first time.

Topics & Concepts

RadioluminescencePhotoluminescenceAnalytical Chemistry (journal)Materials scienceLuminescenceDysprosiumEmission spectrumDopingPhosphorScintillatorQuenching (fluorescence)Spectral lineFluorescenceOpticsChemistryPhysicsOptoelectronicsAstronomyInorganic chemistryDetectorChromatographyGlass properties and applicationsLuminescence Properties of Advanced MaterialsNuclear materials and radiation effects