A Mo–salicylaldehyde-linker (Mo–Tp) based 2D MOF as a single-atom catalyst for the nitrogen reduction reaction
Hassan A. Alhadidi Almheiri, Nirpendra Singh, Dinesh Shetty, Kyriaki Polychronopoulou, Ali A. AlHammadi
Abstract
This work investigates a Mo–Tp 2D MOF screened from a number of different transition-metal-based 2D MOFs. After exfoliation, the Mo–Tp 2D MOF produces ammonia via the distal pathway at a very low limiting potential of −0.38 V.
Topics & Concepts
SalicylaldehydeCatalysisLinkerTransition metalNitrogenAtom (system on chip)Reduction (mathematics)ChemistryNitrogen atomLimitingMaterials scienceCombinatorial chemistryStereochemistryOrganic chemistryRing (chemistry)Schiff baseGeometryOperating systemMathematicsMechanical engineeringComputer scienceEngineeringEmbedded systemAmmonia Synthesis and Nitrogen ReductionMXene and MAX Phase MaterialsAdvanced Photocatalysis Techniques