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Nanosecond X-ray photon correlation spectroscopy using pulse time structure of a storage-ring source

Wonhyuk Jo, Fabian Westermeier, Rustam Rysov, O. Leupold, Florian Schulz, Steffen Tober, Verena Markmann, Michael Sprung, Allesandro Ricci, Torsten Laurus, A. Allahgholi, A. Klyuev, U. Trunk, H. Graafsma, G. Grübel, Wojciech Roseker

2020IUCrJ23 citationsDOIOpen Access PDF

Abstract

X-ray photon correlation spectroscopy (XPCS) is a routine technique to study slow dynamics in complex systems at storage-ring sources. Achieving nanosecond time resolution with the conventional XPCS technique is, however, still an experimentally challenging task requiring fast detectors and sufficient photon flux. Here, the result of a nanosecond XPCS study of fast colloidal dynamics is shown by employing an adaptive gain integrating pixel detector (AGIPD) operated at frame rates of the intrinsic pulse structure of the storage ring. Correlation functions from single-pulse speckle patterns with the shortest correlation time of 192 ns have been calculated. These studies provide an important step towards routine fast XPCS studies at storage rings.

Topics & Concepts

NanosecondDetectorDynamic light scatteringStorage ringSpectroscopyPulse (music)AutocorrelationPhysicsPhotonOpticsMaterials scienceNanotechnologyLaserMathematicsNanoparticleStatisticsBeam (structure)Quantum mechanicsX-ray Spectroscopy and Fluorescence AnalysisAdvanced X-ray Imaging TechniquesSpectroscopy and Quantum Chemical Studies