Litcius/Paper detail

Palladium Catalyzed Dicarbonylation of α-Iodo-Substituted Alkylidenecyclopropanes: Synthesis of Carbamoyl Substituted Indenones

Lin Li, Xin‐Lian Liu, Jin-Yan Liang, Yong-Yu He, Ai‐Jun Ma, Wei-Feng Wang, Jin‐Bao Peng

2022Organic Letters20 citationsDOI

Abstract

A palladium catalyzed dicarbonylation of α-iodo-substituted ACPs for the synthesis of carbamoyl substituted indenones has been developed. Two carbonyl groups were incorporated into the product with the cleavage of the proximal C-C bond of the ACPs. A broad range of carbamoyl substituted indenones were efficiently prepared in good to excellent yields.

Topics & Concepts

ChemistryPalladiumCatalysisCleavage (geology)Combinatorial chemistryBond cleavageMedicinal chemistryOrganic chemistryEngineeringFracture (geology)Geotechnical engineeringCyclopropane Reaction MechanismsCatalytic Alkyne ReactionsCatalytic C–H Functionalization Methods