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Tailoring the stability of a two-color, two-photon rubidium frequency standard

Emily J. Ahern, Sarah K. Scholten, Clayton R. Locke, Nicolas Bourbeau Hébert, Benjamin W. White, André N. Luiten, Christopher Perrella

2025Physical Review Applied11 citationsDOI

Abstract

Rubidium two-photon frequency standards are emerging as powerful contenders for compact, durable devices with exceptional stability. To date, the field has focused on single-color excitation; here, we demonstrate the key advantages of a two-color excitation of a two-photon optical frequency standard based on the $5{S}_{1/2}\ensuremath{\rightarrow}5{D}_{5/2}$ transition of rubidium-87 using driving fields at 780 and 776 nm. Using the $5{P}_{3/2}$ intermediate state to resonantly enhance the transition, we show that frequency stabilities comparable to rubidium single-color two-photon frequency standards can be attained, notably with approximately tenfold lower optical power and tenfold lower rubidium vapor density. Optimization of the detuning from the $5{P}_{3/2}$ intermediate state and of the optical powers of the driving lasers has a dramatic effect on the frequency stability, achieving the best short-term stability of any two-photon rubidium frequency standard to date: $6\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}14}$ at $\ensuremath{\tau}=1$ s. We demonstrate that this level of performance is compatible with a compact geometry by fully self-referencing the frequency standard using an integrated fiber frequency comb to simultaneously stabilize the 780-nm laser's detuning from the $5{P}_{3/2}$ intermediate state, producing a frequency-stable microwave output. A comprehensive noise characterization underpins our observations of this two-color frequency standard, explaining the measured stability and showing that this frequency standard is initially shot-noise limited before becoming limited by light shifts in the long term. This work represents a major advance toward a low size, weight, and power frequency standard based on two-color excitation.

Topics & Concepts

RubidiumStability (learning theory)PhotonPhysicsOpticsMaterials scienceComputer scienceMachine learningMetallurgyPotassiumAtomic and Subatomic Physics ResearchAdvanced Frequency and Time StandardsSpectroscopy and Laser Applications
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