Gate-Switchable Arrays of Quantum Light Emitters in Contacted Monolayer MoS<sub>2</sub> van der Waals Heterodevices
Alexander Hötger, Julian Klein, Katja Barthelmi, Lukas Sigl, Florian Sigger, W. Männer, Samuel Gyger, Matthias Florian, Michael Lorke, F. Jahnke, Takashi Taniguchi, Kenji Watanabe, Klaus D. Jöns, Ursula Wurstbauer, Christoph Kastl, Kai Müller, Jonathan J. Finley, Alexander W. Holleitner
Abstract
We demonstrate electrostatic switching of individual, site-selectively generated matrices of single photon emitters (SPEs) in MoS2 van der Waals heterodevices. We contact monolayers of MoS2 in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom gates. After the assembly of such gate-tunable heterodevices, we demonstrate how arrays of defects, that serve as quantum emitters, can be site-selectively generated in the monolayer MoS2 by focused helium ion irradiation. The SPEs are sensitive to the charge carrier concentration in the MoS2 and switch on and off similar to the neutral exciton in MoS2 for moderate electron doping. The demonstrated scheme is a first step for producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS2 heterostacks.