Litcius/Paper detail

Probing thermoelectric properties of high potential Ca<sub>3</sub>PbO: An Ab Initio Study

Tavneet Kaur, M.M. Sinha

2021IOP Conference Series Materials Science and Engineering12 citationsDOIOpen Access PDF

Abstract

Abstract The fascinating electron transport properties of anti-perovskites have gathered incredible research consideration. In the search for novel thermoelectric materials, a Density Functional Theory (DFT) based computational assessment of electron transport properties of Ca 3 PbO has been made based on the grounds of Boltzmann transport theory. The variation of transport properties specifically Seeback coefficient (S), electrical conductivity (σ), electronic thermal conductivity (κ e ) and power factor (P F ) versus chemical potential (µ) have been plotted at 300 K, 600 K and 800 K. The present study proposes Ca 3 PbO to be an excellent n-type high temperature thermoelectric material. The optimized values of equilibrium structural parameters have been determined. The current analysis tends to stimulate experimental work towards designing and improving thermoelectric performance of Ca 3 PbO for realistic applications.

Topics & Concepts

Thermoelectric effectSeebeck coefficientBoltzmann constantThermoelectric materialsDensity functional theoryThermal conductivityMaterials scienceTransport theoryAb initioWork (physics)ThermodynamicsElectron transport chainElectrical resistivity and conductivityBoltzmann equationCondensed matter physicsComputational chemistryChemistryStatistical physicsPhysicsQuantum mechanicsBiochemistryOrganic chemistryAdvanced Thermoelectric Materials and DevicesTopological Materials and PhenomenaHeusler alloys: electronic and magnetic properties