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Ultracold Electrons via Near-Threshold Photoemission from Single-Crystal Cu(100)

Siddharth Karkare, Gowri Adhikari, W. Andreas Schroeder, J. K. Nangoi, T. A. Arias, Jared Maxson, H. A. Padmore

2020Physical Review Letters59 citationsDOIOpen Access PDF

Abstract

Achieving a low mean transverse energy or temperature of electrons emitted from the photocathode-based electron sources is critical to the development of next-generation and compact x-ray free electron lasers and ultrafast electron diffraction, spectroscopy, and microscopy experiments. In this Letter, we demonstrate a record low mean transverse energy of 5 meV from the cryo-cooled (100) surface of copper using near-threshold photoemission. Further, we also show that the electron energy spread obtained from such a surface is less than 11.5 meV, making it the smallest energy spread electron source known to date: more than an order of magnitude smaller than any existing photoemission, field emission, or thermionic emission based electron source. Our measurements also shed light on the physics of electron emission and show how the energy spread at few meV scale energies is limited by both the temperature and the vacuum density of states.

Topics & Concepts

Thermionic emissionElectronAtomic physicsPhotocathodePhysicsInverse photoemission spectroscopyReflection high-energy electron diffractionAngle-resolved photoemission spectroscopyField electron emissionUltrafast electron diffractionMaterials scienceElectron diffractionLaserUltrashort pulseDiffractionCondensed matter physicsOpticsElectronic structureNuclear physicsAdvanced Electron Microscopy Techniques and ApplicationsElectron and X-Ray Spectroscopy TechniquesPhotocathodes and Microchannel Plates