Litcius/Paper detail

Electron Wave Packet Interference in Atomic Inner-Shell Excitation

T. Kaneyasu, Y. Hikosaka, Masaki Fujimoto, Hiroshi Iwayama, Masahiro Katoh

2021Physical Review Letters18 citationsDOI

Abstract

We report the observation of quantum interference between electron wave packets launched from the inner-shell 4d orbital of the Xe atom. Using pairs of femtosecond radiation wave packets from a synchrotron light source, we obtain time-domain interferograms for the inner-shell excitations. This approach enables the experimental verification and control of the quantum interference between the electron wave packets. Furthermore, the femtosecond Auger decay of the inner-shell excited state is tracked. To the best of our knowledge, this is the first observation of wave packet interference in an atomic inner-shell process, and also the first time-resolved experiment on few-femtosecond Auger decay using a synchrotron light source.

Topics & Concepts

Wave packetAtomic physicsFemtosecondPhysicsSynchrotron radiationExcited stateElectronInterference (communication)ExcitationAtomic orbitalLaserOpticsNuclear physicsQuantum mechanicsEngineeringElectrical engineeringChannel (broadcasting)Laser-Matter Interactions and ApplicationsAdvanced Chemical Physics StudiesSpectroscopy and Quantum Chemical Studies
Electron Wave Packet Interference in Atomic Inner-Shell Excitation | Litcius