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Ketone-functionalized conjugated organic polymers boost red-light-driven molecular oxygen-mediated oxygenation

Hao Zhang, Tingting Yuan, Nursaya Zhumabay, Zhipeng Ruan, Hai Qian, Magnus Rueping

2024Chemical Science10 citationsDOIOpen Access PDF

Abstract

as a green oxidant under 640 nm light irradiation, achieving high yield in short reaction times. Detailed mechanistic investigations clearly showed the role of oxygen and the photocatalyst. This work provides valuable insights into the potential of ketone-modified POPs for superior photocatalytic activation of molecular oxygen under low-energy light conditions.

Topics & Concepts

Conjugated systemOxygenationPolymerKetoneMolecular oxygenOxygenChemistryPhotochemistryPolymer chemistryCombinatorial chemistryOrganic chemistryEcologyBiologyRadical Photochemical ReactionsOxidative Organic Chemistry ReactionsLuminescence and Fluorescent Materials
Ketone-functionalized conjugated organic polymers boost red-light-driven molecular oxygen-mediated oxygenation | Litcius