Litcius/Paper detail

Multigas Sensing Technique Based on Quartz Crystal Tuning Fork-Enhanced Laser Spectroscopy

Linguang Xu, Sheng Zhou, Ningwu Liu, Minghui Zhang, Jingqiu Liang, Jingsong Li

2020Analytical Chemistry149 citationsDOI

Abstract

A compact multigas sensor system based on a single quartz crystal tuning fork (QCTF) and multifrequency synchronous modulation strategy is proposed for trace gas detection. To demonstrate the novel detection technique, three near-infrared continuous-wave (CW) distributed feedback (DFB) diode lasers with center wavelengths of near 1391, 1574, and 1653 nm and a standard 32 kHz QCTF were integrated for simultaneous detection of H2O, CO2, and CH4, respectively. Wavelength modulation spectroscopy with second harmonic detection (WMS-2f) was selected for enhancing sensitivity. Design of the sensor configuration and primary performance between the traditional single-frequency modulation and the proposed tri-frequency modulation were experimentally investigated and compared in detail. The results indicate that the proposed sensing technique has significant advantages of cost effectiveness, portability, and ease-of-use, and detection limits of 1.4, 353, and 3.1 ppm for simultaneously measuring H2O, CO2, and CH4, respectively, are obtained, corresponding to the normalized noise equivalent absorption (NNEA) coefficients of 2.65 × 10–10, 8.09 × 10–10, and 8.28 × 10–10 cm–1 W/√Hz, respectively. Moreover, the use of an erbium-doped fiber amplifier (EDFA) has been demonstrated as an effective method for sensitivity enhancement.

Topics & Concepts

LaserChemistrySpectroscopyWavelengthSensitivity (control systems)Modulation (music)DiodeAmplifierOpticsOptoelectronicsCrystal (programming language)Materials scienceElectronic engineeringPhysicsComputer scienceAcousticsProgramming languageQuantum mechanicsEngineeringCMOSSpectroscopy and Laser ApplicationsGas Sensing Nanomaterials and SensorsAtmospheric Ozone and Climate
Multigas Sensing Technique Based on Quartz Crystal Tuning Fork-Enhanced Laser Spectroscopy | Litcius