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Comparative study on two imidazolium‐based ionic liquid surfactants as corrosion inhibitors for N80 steel in 15% hydrochloric acid solution

Kangquan Qiao, Ying Zeng

2020Materials and Corrosion26 citationsDOI

Abstract

Abstract A comparative study on 1‐dodecyl‐2,3‐dimethylimidazolium chloride ([DDMIM]Cl) and 1‐benzyl‐3‐dodecyl‐2‐methylimidazol‐1‐ium chloride ([BDMIM]Cl) as corrosion inhibitors for N80 steel in a 15% hydrochloric acid solution was performed by surface tension tests, electrochemical measurements, weight loss, scanning electron microscopy, atomic force microscopy, and theoretical calculations. The experimental results confirm that [DDMIM]Cl and [BDMIM]Cl act as mixed‐type inhibitors. The adsorption of both inhibitors on the N80 steel surface obeys the Langmuir adsorption isotherm, and [BDMIM]Cl exhibits better inhibitive performance, lower critical micelle concentration (CMC), and a lower ratio of saturation adsorption concentration on the steel surface to its own CMC than [DDMIM]Cl. The results of theoretical calculations reveal that the electron‐donating/accepting capacities and hydrophobicity of the benzyl substituent in the imidazole ring are essential for preventing steel corrosion in acid media.

Topics & Concepts

Hydrochloric acidAdsorptionCorrosionCritical micelle concentrationIonic liquidImidazoleChlorideSubstituentChemistryBenzyl chlorideElectrochemistryScanning electron microscopeSurface tensionLangmuir adsorption modelInorganic chemistryMicelleNuclear chemistryMaterials scienceOrganic chemistryAqueous solutionCatalysisPhysical chemistryComposite materialElectrodeQuantum mechanicsPhysicsCorrosion Behavior and InhibitionConcrete Corrosion and DurabilityHydrogen embrittlement and corrosion behaviors in metals
Comparative study on two imidazolium‐based ionic liquid surfactants as corrosion inhibitors for N80 steel in 15% hydrochloric acid solution | Litcius