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Catalyst-free, visible-light-promoted S–H insertion reaction between thiols and α-diazoesters

Jingya Yang, Ganggang Wang, Shuwen Chen, Ben Ma, Hongyan Zhou, Menghui Song, Cai Liu, Congde Huo

2020Organic & Biomolecular Chemistry33 citationsDOI

Abstract

A visible-light-promoted S-H insertion reaction between thiols and α-diazoesters was developed. The reaction proceeded smoothly at room temperature with a broad substrate scope, affording various thioethers in moderate to excellent yields. The catalyst- and additive-free nature, sustainable energy source and mild reaction conditions make this strategy more eco-friendly.

Topics & Concepts

ChemistryCatalysisPhotochemistryVisible spectrumInsertion reactionCombinatorial chemistryMedicinal chemistryOrganic chemistryPhysicsOptoelectronicsCyclopropane Reaction MechanismsSulfur-Based Synthesis TechniquesCatalytic C–H Functionalization Methods
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