Out-of-plane trion emission in monolayer WSe2 revealed by whispering gallery modes of dielectric microresonators
Daniel Andres‐Penares, Mojtaba Karimi Hábil, Alejandro Molina‐Sánchez, Carlos J. Zapata-Rodrı́guez, Juan P. Martínez‐Pastor, Juan F. Sánchez‐Royo
Abstract
Abstract The manipulation of light emitted by two-dimensional semiconductors grounds forthcoming technologies in the field of on-chip communications. However, these technologies require from the so elusive out-of-plane photon sources to achieve an efficient coupling of radiated light into planar devices. Here we propose a versatile spectroscopic method that enables the identification of the out-of-plane component of dipoles. The method is based on the selective coupling of light emitted by in-plane and out-of-plane dipoles to the whispering gallery modes of spherical dielectric microresonators, in close contact to them. We have applied this method to demonstrate the existence of dipoles with an out-of-plane orientation in monolayer WSe 2 at room temperature. Micro-photoluminescent measurements, numerical simulations based on finite element methods, and ab-initio calculations have identified trions as the source responsible for this out-of-plane emission, opening new routes for realizing on-chip integrated systems with applications in information processing and quantum communications.