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Silver-catalyzed cyclopropanation of alkenes with alkynyl <i>N</i>-nosylhydrazones leading to alkynyl cyclopropanes

Yongquan Ning, Mengtian Huo, Lizuo Wu, Xihe Bi

2022Chemical Communications18 citationsDOI

Abstract

-nosylhydrazones as alkynyl carbene precursors, is reported. This method provides a straightforward and powerful approach for preparing various alkynyl cyclopropanes in high yield with excellent stereoselectivities. In addition, the practicality of this method was demonstrated by gram-scale synthesis and late-stage modification of bioactive molecules.

Topics & Concepts

CyclopropanationCarbeneYield (engineering)ChemistryCatalysisStereoselectivityCombinatorial chemistryOrganic chemistryMaterials scienceMetallurgyCyclopropane Reaction MechanismsCatalytic Alkyne ReactionsCatalytic C–H Functionalization Methods
Silver-catalyzed cyclopropanation of alkenes with alkynyl <i>N</i>-nosylhydrazones leading to alkynyl cyclopropanes | Litcius