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Soft X-ray ARPES for three-dimensional crystals in the micrometre region

Takayuki Muro, Yasunori Senba, Haruhiko Ohashi, Takuo Ohkochi, T. Matsushita, T. Kinoshita, Shik Shin

2021Journal of Synchrotron Radiation22 citationsDOIOpen Access PDF

Abstract

An endstation dedicated to angle-resolved photoemission spectroscopy (ARPES) using a soft X-ray microbeam has been developed at the beamline BL25SU of SPring-8. To obtain a high photoemission intensity, this endstation is optimized for measurements under the condition of grazing beam incidence to a sample surface, where the glancing angle is 5° or smaller. A Wolter mirror is used for focusing the soft X-rays. Even at the glancing angle of 5°, the smallest beam spot still having a sufficient photon flux for ARPES is almost round on the sample surface and the FWHM diameter is ∼5 µm. There is no need to change the sample orientation for performing k x − k y mapping by virtue of the electron lens with a deflector of the photoelectron analyzer, which makes it possible to keep the irradiation area unchanged. A partially cleaved surface area as small as ∼20 µm was made on an Si(111) wafer and ARPES measurements were performed. The results are presented.

Topics & Concepts

Angle-resolved photoemission spectroscopyOpticsBeamlineMicrobeamMaterials scienceX-ray photoelectron spectroscopyPhotoemission spectroscopyMonochromatorSynchrotronPhysicsBeam (structure)Nuclear magnetic resonanceCondensed matter physicsElectronic structureWavelengthElectron and X-Ray Spectroscopy TechniquesX-ray Spectroscopy and Fluorescence AnalysisAdvanced Electron Microscopy Techniques and Applications