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Spin–valley protected Kramers pair in bilayer graphene

Artem O. Denisov, Veronika Reckova, Solenn Cances, Max J. Ruckriegel, Michele Masseroni, Christoph Adam, Chuyao Tong, Jonas D. Gerber, W. Huang, Kenji Watanabe, Takashi Taniguchi, Thomas Ihn, K. Ensslin, Hadrien Duprez

2025Nature Nanotechnology19 citationsDOIOpen Access PDF

Abstract

The intrinsic valley degree of freedom makes bilayer graphene (BLG) a unique platform for semiconductor qubits. The single-carrier quantum dot (QD) ground state exhibits a twofold degeneracy, where the two states that constitute a Kramers pair have opposite spin and valley quantum numbers. Because of the valley-dependent Berry curvature, an out-of-plane magnetic field breaks the time-reversal symmetry of this ground state and a qubit can be encoded in the spin-valley subspace. The Kramers states are protected against known spin- and valley-mixing mechanisms because mixing requires a simultaneous change of the two quantum numbers. Here, we fabricate a tunable QD device in Bernal BLG and measure a spin-valley relaxation time for the Kramers states of 38 s at 30 mK, which is two orders of magnitude longer than the 0.4 s measured for purely spin-blocked states. We also show that the intrinsic Kane-Mele spin-orbit splitting enables a Kramers doublet single-shot readout even at zero magnetic field with a fidelity above 99%. If these long-lived Kramers states also possess long coherence times and can be effectively manipulated, electrostatically defined QDs in BLG may serve as long-lived semiconductor qubits, extending beyond the spin qubit paradigm.

Topics & Concepts

PhysicsCondensed matter physicsQubitSpin (aerodynamics)Quantum mechanicsGround stateSpin statesSpin engineeringQuantum dotQuantumSpin polarizationThermodynamicsElectronQuantum and electron transport phenomenaGraphene research and applicationsTopological Materials and Phenomena
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