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Dual-comb spectroscopy in the deep ultraviolet

John J. McCauley, Mark C. Phillips, Reagan R. D. Weeks, Yu Zhang, S. S. Harilal, R. Jason Jones

2024Optica25 citationsDOIOpen Access PDF

Abstract

This Letter reports dual-frequency-comb spectroscopy in the deep ultraviolet used to characterize transient laser-produced plasmas. Dual-comb spectroscopy at these wavelengths enables access to a large number of strong electronic transitions in neutral and ionized atoms and molecules. This broadband dual-frequency-comb system at 265 nm measures multiple transitions in neutral and singly ionized iron atoms in a laser-produced plasma. Analysis of absorption spectra yields time-resolved ion and neutral column densities, excitation temperatures, and electron densities, which are measured down to 10 14 cm −3 levels. The results provide insights into low-temperature plasma properties.

Topics & Concepts

SpectroscopyIonizationPlasmaAtomic physicsAbsorption spectroscopyIonLaserSpectral lineExcitationUltravioletAbsorption (acoustics)Materials scienceAtomic electron transitionChemistryOpticsOptoelectronicsPhysicsOrganic chemistryAstronomyQuantum mechanicsComposite materialLaser-induced spectroscopy and plasmaAtomic and Molecular PhysicsMass Spectrometry Techniques and Applications
Dual-comb spectroscopy in the deep ultraviolet | Litcius