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Assessment of a subgrid‐scale model for convection‐dominated mass transfer for initial transient rise of a bubble

Andre Weiner, Claire M.Y. Claassen, Irian R. Hierck, J.A.M. Kuipers, M.W. Baltussen

2022AIChE Journal15 citationsDOIOpen Access PDF

Abstract

Abstract The mass transfer between a rising bubble and the surrounding liquid is mainly determined by an extremely thin layer of dissolved gas near the bubble interface. Resolving this concentration boundary layer in numerical simulations is computationally expensive and limited to low Péclet numbers. Subgrid‐scale (SGS) models mitigate the resolution requirements by approximating the mass transfer near the interface. In this contribution, we validate an improved SGS model with a single‐phase simulation approach, which solves only the liquid phase at a highly resolved mesh. The mass transfer during the initial transient rise of moderately deformed bubbles in the range Re = 72–569 and Sc = 10 2 –10 4 is carefully validated. The single‐phase approach is able to mirror the two‐phase flow field. The time‐dependent local and global mass transfer of both approaches agree well. The difference in the global Sherwood number is below than 2.5%. The improved SGS model predicts the mass transfer accurately and shows marginal mesh dependency.

Topics & Concepts

Mass transferBubbleMechanicsTransient (computer programming)Sherwood numberBoundary layerScale (ratio)Phase (matter)Flow (mathematics)Mass transfer coefficientConvectionTwo-phase flowChemistryPhysicsComputer scienceOperating systemQuantum mechanicsTurbulenceOrganic chemistryNusselt numberReynolds numberFluid Dynamics and Heat TransferFluid Dynamics and MixingLattice Boltzmann Simulation Studies
Assessment of a subgrid‐scale model for convection‐dominated mass transfer for initial transient rise of a bubble | Litcius