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A High Throughput Aqueous Passivation Testing Methodology for Compositionally Complex Alloys Using a Scanning Droplet Cell

Debashish Sur, Howie Joress, Jason Hattrick‐Simpers, John R. Scully

2023Journal of The Electrochemical Society20 citationsDOIOpen Access PDF

Abstract

Compositionally complex alloys containing four or more principal elements provide an opportunity to explore a wide range of compositions, processing, and microstructural variables to find new materials with unique properties. In particular, the discovery of novel alloys that form self-healing, protective passivating films is of substantial interest. Probing experimentally a robust landscape of such alloys requires the utilization of high-throughput electrochemical methods to uncover key differences, ideally captured by discriminating metrics, indicative of superior properties. Herein, a methodology is demonstrated using a scanning droplet cell for a rapid passivation behavior evaluation of Al 0.7-x-y Co x Cr y Fe 0.15 Ni 0.15 combinatorial alloy library in 0.1 mol l −1 H 2 SO 4(aq) .

Topics & Concepts

PassivationAlloyThroughputMaterials scienceElectrochemistryScanning electron microscopeNanotechnologyChemical engineeringMetallurgyComputer scienceChemistryComposite materialElectrodePhysical chemistryEngineeringTelecommunicationsLayer (electronics)WirelessElectrocatalysts for Energy ConversionMachine Learning in Materials ScienceAdvanced Memory and Neural Computing