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Nanopores of a Covalent Organic Framework: A Customizable Vessel for Organocatalysis

Debanjan Chakraborty, Dinesh Mullangi, Chandana Chandran, Ramanathan Vaidhyanathan

2022ACS Omega32 citationsDOIOpen Access PDF

Abstract

utilization, and more complex biomimetic catalysis. Such catalysts employ COF as a "passive" support that merely docks catalytically active inorganic clusters, or in other cases, the COF itself participates as an "active" support by altering the electronics of the inorganic catalytic sites through the redox activity of its framework. Even more, catalytic organic pockets or metal complexes have been directly tethered to COF walls to make them behave like single-site organocatalysts. Here, we have listed most COF-based organic transformations by categorizing them as metal-free non-noble-metal@COF and noble-metal@COF. The initial part of this review highlights the advantages of COFs as a component of a heterogeneous catalyst, while the latter part discusses all of the current literature on this topic.

Topics & Concepts

Covalent organic frameworkCatalysisKnoevenagel condensationCovalent bondNoble metalHeterogeneous catalysisOrganocatalysisMaterials scienceMetal-organic frameworkNanotechnologyChemistryChemical engineeringOrganic chemistryAdsorptionEnantioselective synthesisEngineeringCovalent Organic Framework ApplicationsMetal-Organic Frameworks: Synthesis and ApplicationsLuminescence and Fluorescent Materials
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