Litcius/Paper detail

Catalytic charge transfer complex enabled difluoromethylation of enamides with difluoromethyltriphenylphosphonium bromide

Ping Li, Qiang Liu, Dequn Sun, Xiang‐Yu Chen

2022Organic & Biomolecular Chemistry15 citationsDOI

Abstract

A catalytic charge transfer complex strategy that enabled difluoromethylation and ethoxycarbonylmonofluoromethylation of enamides with phosphonium bromine salts has been reported. This strategy also provides a convenient approach for the synthesis of functionalized oxindoles and 1,1-diphenylethylenes with easily available phosphonium bromine salts and a catalytic amount of iodine anion.

Topics & Concepts

PhosphoniumChemistryBromineBromideCatalysisCombinatorial chemistryPhosphonium saltIodineOrganic chemistryFluorine in Organic ChemistryCatalytic C–H Functionalization MethodsSynthesis and Catalytic Reactions