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High-frequency rectification via chiral Bloch electrons

Hiroki Isobe, Su-Yang Xu, Liang Fu

2020Science Advances205 citationsDOIOpen Access PDF

Abstract

Rectification is a process that converts electromagnetic fields into a direct current. Such a process underlies a wide range of technologies such as wireless communication, wireless charging, energy harvesting, and infrared detection. Existing rectifiers are mostly based on semiconductor diodes, with limited applicability to small-voltage or high-frequency inputs. Here, we present an alternative approach to current rectification that uses the intrinsic electronic properties of quantum crystals without using semiconductor junctions. We identify a previously unknown mechanism for rectification from skew scattering due to the inherent chirality of itinerant electrons in time-reversal invariant but inversion-breaking materials. Our calculations reveal large, tunable rectification effects in graphene multilayers and transition metal dichalcogenides. Our work demonstrates the possibility of realizing high-frequency rectifiers by rational material design and quantum wave function engineering.

Topics & Concepts

RectificationSkewElectronQuantumSemiconductorPhysicsWave functionOptical rectificationScatteringWork (physics)DiodeChirality (physics)Coherence (philosophical gambling strategy)OptoelectronicsSchottky diodeGrapheneElectromagnetic radiationInfraredDegrees of freedom (physics and chemistry)Work functionFunction (biology)Quantum mechanicsRational designGravitational singularityInvariant (physics)Semiconductor deviceRectifier (neural networks)Topological Materials and PhenomenaQuantum and electron transport phenomenaStrong Light-Matter Interactions
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