Recent Advancements and Perspectives of Low-Dimensional Halide Perovskites for Visual Perception and Optoelectronic Applications
Hummera Rafique, Ghulam Abbas, Manuel J. Mendes, Pedro Barquinha, Rodrigo Martins, Elvira Fortunato, Hugo Águas, Santanu Jana
Abstract
Low-dimensional (LD) halide perovskites have attracted considerable attention due to their distinctive structures and exceptional optoelectronic properties, including high absorption coefficients, extended charge carrier diffusion lengths, suppressed non-radiative recombination rates, and intense photoluminescence. A key advantage of LD perovskites is the tunability of their optical and electronic properties through the precise optimization of their structural arrangements and dimensionality. This review systematically examines recent progress in the synthesis and optoelectronic characterizations of LD perovskites, focusing on their structural, optical, and photophysical properties that underpin their versatility in diverse applications. The review further summarizes advancements in LD perovskite-based devices, including resistive memory, artificial synapses, photodetectors, light-emitting diodes, and solar cells. Finally, the challenges associated with stability, scalability, and integration, as well as future prospects, are discussed, emphasizing the potential of LD perovskites to drive breakthroughs in device efficiency and industrial applicability.