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Anomalous transport in high-mobility superconducting SrTiO <sub>3</sub> thin films

Jin Yue, Yilikal Ayino, Tristan K. Truttmann, Maria N. Gastiasoro, Eylon Persky, Alex Khanukov, Dooyong Lee, Laxman Raju Thoutam, Beena Kalisky, Rafael M. Fernandes, Vlad Pribiag, Bharat Jalan

2022Science Advances13 citationsDOIOpen Access PDF

Abstract

The study of subtle effects on transport in semiconductors requires high-quality epitaxial structures with low defect density. Using hybrid molecular beam epitaxy (MBE), SrTiO 3 films with a low-temperature mobility exceeding 42,000 cm 2 V −1 s −1 at a low carrier density of 3 × 10 17 cm −3 were achieved. A sudden and sharp decrease in residual resistivity accompanied by an enhancement in the superconducting transition temperature were observed across the second Lifshitz transition where the third band becomes occupied, revealing dominant intraband scattering. These films further revealed an anomalous behavior in the Hall carrier density as a consequence of the antiferrodistortive (AFD) transition and the temperature dependence of the Hall scattering factor. Using hybrid MBE growth, phenomenological modeling, temperature-dependent transport measurements, and scanning superconducting quantum interference device imaging, we provide critical insights into the important role of inter- versus intraband scattering and of AFD domain walls on normal-state and superconducting properties of SrTiO 3 .

Topics & Concepts

Condensed matter physicsScatteringMolecular beam epitaxySuperconductivityResidual resistivityHall effectMaterials scienceElectrical resistivity and conductivityElectron mobilitySemiconductorEpitaxyScattering ratePhysicsOptoelectronicsNanotechnologyOpticsLayer (electronics)Quantum mechanicsElectronic and Structural Properties of OxidesMagnetic and transport properties of perovskites and related materialsSemiconductor materials and devices
Anomalous transport in high-mobility superconducting SrTiO <sub>3</sub> thin films | Litcius