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Synthesis of Tetrahydroquinolines via Borrowing Hydrogen Methodology Using a Manganese PN<sup>3</sup> Pincer Catalyst

Natalie Hofmann, Leonard Homberg, Kai C. Hultzsch

2020Organic Letters32 citationsDOIOpen Access PDF

Abstract

pincer complex. The reaction selectively leads to 1,2,3,4-tetrahydroquinolines thanks to a targeted choice of base. This strategy provides an atom-efficient pathway with water as the only byproduct. In addition, no further reducing agents are required.

Topics & Concepts

ChemistryPincer movementCatalysisManganeseCombinatorial chemistryCascade reactionCascadeHydrogenBase (topology)Organic chemistryMathematicsMathematical analysisChromatographyAsymmetric Hydrogenation and CatalysisChemical Synthesis and AnalysisNanomaterials for catalytic reactions
Synthesis of Tetrahydroquinolines via Borrowing Hydrogen Methodology Using a Manganese PN<sup>3</sup> Pincer Catalyst | Litcius