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<i>Ab-Initio</i> Calculations of Oxygen Vacancy in Ga <sub>2</sub> O <sub>3</sub> Crystals

А. Usseinov, Zh. Koishybayeva, Alexander Platonenko, А. Аkilbekov, J. Purāns, Vladimir Pankratov, Yana Suchikova, Anatoli I. Popov

2021Latvian Journal of Physics and Technical Sciences21 citationsDOIOpen Access PDF

Abstract

Abstract Gallium oxide β-Ga 2 O 3 is an important wide-band gap semiconductor. In this study, we have calculated the formation energy and transition levels of oxygen vacancies in β-Ga 2 O 3 crystal using the B3LYP hybrid exchange-correlation functional within the LCAO-DFT approach. The obtained electronic charge redistribution in perfect Ga 2 O 3 shows notable covalency of the Ga-O bonds. The formation of the neutral oxygen vacancy in β-Ga 2 O 3 leads to the presence of deep donor defects with quite low concentration. This is a clear reason why oxygen vacancies can be hardly responsible for n-type conductivity in β-Ga 2 O 3 .

Topics & Concepts

GalliumVacancy defectOxygenHybrid functionalAb initioMaterials scienceBand gapRedistribution (election)Ab initio quantum chemistry methodsCrystallographySemiconductorDensity functional theoryCondensed matter physicsComputational chemistryChemistryPhysicsMoleculeOptoelectronicsOrganic chemistryLawMetallurgyPoliticsPolitical scienceGa2O3 and related materialsZnO doping and propertiesAdvanced Photocatalysis Techniques