Litcius/Paper detail

A study of the temperature effect on the spray characteristics in the cone-jet mode of electrohydrodynamic atomization (EHDA) with viscous liquids

Hailong Liu, Honglei Wu, Yang Ding, Jiaqi Chen, Junfeng Wang

2023Physics of Fluids11 citationsDOI

Abstract

In this work, the near-field spray characteristics of electrohydrodynamic atomization (EHDA) for viscous liquids (ethanol, G20, G40, G50, G66, and glycerol) under various temperatures T (T is from 293 to 343 K), electric Bond numbers BoE (BoE is from 0 to 3.5) and dimensionless flow rate Q* (Q* is from 11 to 400) have been investigated by employing a high-speed imaging technique. The transition of the spray modes, variations of the spray angle θ1, semi-angle of Taylor cone θ2, and spraying droplet size (the Sauter mean diameter D32 and the probability density function) in the cone-jet mode have been studied experimentally. The results indicate that the stable cone-jet mode disappeared regardless of increasing BoE for working fluids with relatively higher viscosity (G50, G66, and glycerol). Nevertheless, the temperature elevation promotes the appearance of the stable cone-jet mode, e.g., G66 fluid could form the stable cone-jet as liquid temperature increases to 343 K. Moreover, the temperature plays a significant role in improving the spray angle and the semi-angle of the Taylor cone, as well as droplet size distributions. Specifically, in the case of G40 fluid, the spray angle increased from about 20.8°–23.9° at room temperature (293 K) to around 34.1°–37° at 343 K. Meanwhile, the droplet size distributions were shifting from 9.73–35.49 μm at 293 K to 4.39–23.84 μm at 343 K. The increase in temperature causes a dramatic viscosity reduction in highly viscous fluids, and the viscous dissipation during the atomization reduced substantially. As a result, more kinetic energy was retained to overcome the surface energy and thus improve the quality of the spray. In addition, the dimensionless droplet size D* in the stable cone-jet mode shows a linear scaling relationship with Q*. By introducing an Arrhenius-type equation to account for the temperature effect, a model to predict dimensionless droplet size D* under various dimensionless flow rates Q* and liquid temperatures T has been proposed. The model is in good agreement with the experimental data under the stable cone-jet mode in the EHDA for viscous fluids at a range of temperatures.

Topics & Concepts

ElectrohydrodynamicsJet (fluid)Ligand cone angleDimensionless quantityPhysicsViscositySpray characteristicsSauter mean diameterMechanicsWeber numberWork (physics)Electric fieldThermodynamicsReynolds numberAnalytical Chemistry (journal)Materials scienceChemistryNozzleComposite materialTurbulenceSpray nozzleChromatographyQuantum mechanicsConical surfaceElectrohydrodynamics and Fluid DynamicsFluid Dynamics and Heat TransferMass Spectrometry Techniques and Applications