Litcius/Paper detail

Influence of oxygen and nitrogen doping on the structure and magnetic properties of CoNi alloy: First principle calculations

Abdalla Obeidat, Bilal Aladerah, Mohammad-Khair Qaseer

2022Journal of Physics and Chemistry of Solids23 citationsDOIOpen Access PDF

Abstract

We have studied the effects of oxygen and nitrogen doping as interstitial defects on the structure and magnetic properties of CoNi alloy using the first principle density functional theory , where we include the orbital-spin interaction in the calculations. Our calculations reveal that the CoNi:O Ni in the L1 0 -structure has a large enhancement in the saturation magnetization ( M s ) and a small reduction in the magnetic crystalline anisotropy (MCA). For CoNi:O Co , we found a small reduction in M s and MCA. However, for CoNi:N Co and CoNi:NNi there is always a reduction in M s and MCA. Therefore, the first alloy could be suitable for permanent magnets. A detailed analysis of other parameters, such as the magnetic hardness parameter ( κ ), optimum supercell parameters, anisotropy field ( H a ) , and formation energy ( E f o r ) is presented. The interstitial oxygen doping enhances the magnetic properties .

Topics & Concepts

Density functional theoryCondensed matter physicsAlloyDopingMaterials scienceAnisotropyOxygenMagnetic anisotropySupercellSaturation (graph theory)MagnetMagnetizationMagnetic fieldChemistryComputational chemistryMetallurgyPhysicsOpticsMeteorologyCombinatoricsMathematicsQuantum mechanicsThunderstormOrganic chemistryMagnetic Properties of AlloysMagnetic properties of thin filmsMagnetic and transport properties of perovskites and related materials