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MnO2 nanosheets modified CoP/P-C core/shell nanotubes with vertically aligned channels for promoting supercapacitor performances

Mengjie Pan, Huachen Lin, Lin Sun, Yulong Ying, Hong Jia, Yu Liu

2024Chemical Engineering Science13 citationsDOIOpen Access PDF

Abstract

Research into electrode materials that are low-cost, possess high capacity, and exhibit long cycle life is pivotal for the advancement of supercapacitor technology. Herein, a CoP/P-C/MnO 2 @CC composite is synthesized by solution impregnation and high temperature phosphating. The unique combination of nanotubes and MnO 2 nanosheets reduces ion and electron transmission distance and significantly increases active sites. The CoP/P-C/MnO 2 @CC electrode demonstrates a specific capacitance of 742.0 F g −1 at 1 A g −1 , a substantial improvement over the counterpart prior to KMnO 4 immersion (459.4 F g −1 ). Furthermore, an asymmetric supercapacitor based on the CoP/P-C/MnO 2 @CC electrode was assembled, achieving a high energy density of 93.12 Wh kg −1 at a power density of 800 W kg −1 . Meanwhile, the device maintains 77.3 % of its original capacity after 8000 cycles, demonstrating good cycle stability. This study not only presents an attractive electrode material with unique structure, but also provides a referential methodology for developing superior electrodes.

Topics & Concepts

SupercapacitorMaterials scienceCore (optical fiber)NanotechnologyShell (structure)Chemical engineeringComposite materialChemistryElectrodeCapacitanceEngineeringPhysical chemistrySupercapacitor Materials and FabricationAdvancements in Battery MaterialsElectrocatalysts for Energy Conversion