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Exciton-Trion Polaritons in Doped Two-Dimensional Semiconductors

Farhan Rana, Okan Koksal, Minwoo Jung, Gennady Shvets, A. Nick Vamivakas, Christina Manolatou

2021Physical Review Letters32 citationsDOIOpen Access PDF

Abstract

We present a many-body theory of exciton-trion polaritons (ETPs) in doped two-dimensional semiconductor materials. ETPs are robust coherent hybrid excitations involving excitons, trions, and photons. In ETPs, the 2-body exciton states are coupled to the material ground state via exciton-photon interaction, and the 4-body trion states are coupled to the exciton states via Coulomb interaction. The trion states are not directly optically coupled to the material ground state. The energy-momentum dispersion of ETPs exhibit three bands. We calculate the energy band dispersions and the compositions of ETPs at different doping densities using Green's functions. The energy splittings between the polariton bands, as well as the spectral weights of the polariton bands, depend on the strength of the Coulomb coupling between the excitons and the trions, which in turn depends sensitively on the doping density. The doping density dependence of the ETP bands and the charged nature of the trion states could enable novel electrical and optical control of ETPs.

Topics & Concepts

TrionPolaritonExcitonPhysicsCondensed matter physicsBinding energyExciton-polaritonsAtomic physicsPhotonCoulombDopingBiexcitonGround stateElectronQuantum mechanicsStrong Light-Matter InteractionsPerovskite Materials and ApplicationsPlasmonic and Surface Plasmon Research
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