Litcius/Paper detail

Hollow Waveguide Multipass Cavity Enhanced Raman Spectroscopy for Trace Gases Sensing

Miaolin Wang, Pinyi Wang, Jianxin Wang, T. Liu, Changding Wang, Zhiwei Shen, Weigen Chen

2025Analytical Chemistry8 citationsDOI

Abstract

We report a hollow waveguide multipass cavity (HMC) for enhancing the Raman signal of trace gases. Raman signal collection is improved by a hollow waveguide coated with a multilayer dielectric film on the inner surface. The laser beam is reflected 50 times in the HMC, resulting in an extended interaction length between the laser and gases. The variation between the output Raman signal intensity and the HMC parameters is calculated. The reflection behavior of intracavity beams is also simulated to increase the number of beams. The performance of the HMC apparatus is demonstrated by recording the Raman spectra of ambient air, CH 4, and H 2 . The limits of detection for CH 4 and H 2 are achieved at 0.87 and 2.06 ppm, respectively, with a total pressure of 0.1 MPa and an exposure time of 60 s. Multigas can be detected with high sensitivity using HMC-enhanced Raman spectroscopy, making it a highly promising approach for gas sensing applications.

Topics & Concepts

Raman spectroscopyChemistrySIGNAL (programming language)WaveguideOpticsLaserRaman scatteringReflection (computer programming)DielectricTotal internal reflectionOptoelectronicsSensitivity (control systems)Beam (structure)Analytical Chemistry (journal)SpectroscopyTrace gasCoherent anti-Stokes Raman spectroscopySpectral lineLaser beamsTRACE (psycholinguistics)Raman laserSpectroscopy and Laser ApplicationsPhotonic and Optical DevicesPhotonic Crystal and Fiber Optics