Achieving the selectivity of the oxygen reduction reaction by regulating electron spin states and active centers on Fe–Mn–N<sub>6</sub>–C dual-atom catalysts
Shiyao Li, Honghao Chen, Yue Qiu, Chengxing Cui, Wenhui Zhong, Jun Jiang
Abstract
As the first attempt to reveal the intrinsic relationship between electron spins and catalytic selectivity, this work offers new insights into the rational design of efficient transition metal atom-dispersed catalysts through spin regulation.
Topics & Concepts
SelectivityCatalysisAtom (system on chip)Oxygen reduction reactionSpin statesOxygen atomDual (grammatical number)ElectronOxygenSpin (aerodynamics)ChemistryAtomic physicsReduction (mathematics)Materials scienceInorganic chemistryPhysicsPhysical chemistryMoleculeElectrochemistryElectrodeQuantum mechanicsArtMathematicsGeometryComputer scienceThermodynamicsLiteratureOrganic chemistryEmbedded systemBiochemistryElectrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceFuel Cells and Related Materials