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Synthesis of shape-tunable PbZrTiO<sub>3</sub> nanocrystals with lattice variations for piezoelectric energy harvesting and human motion detection

Ya-Ju Chuang, Arnab Pal, Bo‐Hao Chen, Satyaranjan Jena, Sreerag Suresh, Zong‐Hong Lin, Michael H. Huang

2025Chemical Science13 citationsDOIOpen Access PDF

Abstract

crystals give size- and composition-dependent band gaps. Cuboids show notably larger piezoelectric and ferroelectric responses than cubes. Piezoelectric nanogenerators (PENGs) containing 30 wt% cuboids produce the highest open-circuit voltage of 20.36 V and short-circuit current of 2300 nA. The PENGs harvest energy through bending/releasing cycles to power devices and show photothermal pyroelectric activity. Moreover, a single 30 wt% cuboid PENG device integrated into a shoe insole can deliver an impressive 96.8% accuracy for human motion detection using a machine learning approach. This work illustrates that considerable lattice variation through crystal shape control is effective in enhancing material properties.

Topics & Concepts

NanocrystalPiezoelectricityEnergy harvestingMaterials scienceLattice (music)Human motionNanotechnologyEnergy (signal processing)OptoelectronicsMotion (physics)AcousticsPhysicsComposite materialClassical mechanicsQuantum mechanicsAdvanced Sensor and Energy Harvesting MaterialsConducting polymers and applicationsTactile and Sensory Interactions
Synthesis of shape-tunable PbZrTiO<sub>3</sub> nanocrystals with lattice variations for piezoelectric energy harvesting and human motion detection | Litcius