Rigid two-dimensional indium metal–organic frameworks boosting nitrogen electroreduction at all pH values
Yuntong Sun, Baokai Xia, Shan Ding, Licheng Yu, Sheng Chen, Jingjing Duan
Abstract
Rigid 2D In-MOF nanosheets is investigated as electrocatalysts for nitrogen electroreduction in the entire pH range for the first time, which follows an enzymatic mechanism, with the potential determining step being *H 2 NNH 2 * → *NH 2 + NH 3 .
Topics & Concepts
IndiumNitrogenMetal-organic frameworkChemistryInorganic chemistryMetalBoosting (machine learning)Materials sciencePhysical chemistryOrganic chemistryComputer scienceAdsorptionMachine learningAmmonia Synthesis and Nitrogen ReductionAdvanced Photocatalysis TechniquesMXene and MAX Phase Materials