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Quinoline-Modified Phenanthroline Electron-Transporters as n-Type Exciplex Partners for Highly Efficient and Stable Deep-Red OLEDs

Y. Saito, Hisahiro Sasabe, Hisaki Tsuneyama, Shoki Abe, Misaki Matsuya, Tomoya Kawano, Yuma Kori, Takanori Hanayama, Junji Kido

2023Bulletin of the Chemical Society of Japan13 citationsDOI

Abstract

Abstract Although stable deep-red organic light-emitting devices (OLEDs) exhibit potential applications as unique illumination light sources for plant growth and in health monitoring systems, their electron-to-photon conversion efficiency, represented by the external quantum efficiency (EQE), is significantly lower than that of the other primary colors. Thus, to overcome this limitation, n-type exciplex host partners based on quinoline-modified phenanthroline derivatives, X-BPhen, were designed and synthesized in this study. These X-BPhen derivatives formed exciplexes on combination with a p-type host material, NPD, behaving as host materials in deep-red phosphorescent OLEDs. The corresponding devices exhibited a maximum EQE of 17.6%, with CIE coordinates of (0.71, 0.29), and an LT80 of 410 h at a constant current density of 25 mA/cm2; this is among the best performances reported for stable deep-red OLEDs.

Topics & Concepts

OLEDPhosphorescenceChemistryQuinolineQuantum efficiencyPhenanthrolineExcimerPhotochemistryOptoelectronicsFluorescenceMaterials scienceCrystallographyOpticsOrganic chemistryPhysicsLayer (electronics)Organic Light-Emitting Diodes ResearchLuminescence and Fluorescent MaterialsOrganic Electronics and Photovoltaics
Quinoline-Modified Phenanthroline Electron-Transporters as n-Type Exciplex Partners for Highly Efficient and Stable Deep-Red OLEDs | Litcius