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Single-Step Production of a TiO<sub>2</sub>@MoS<sub>2</sub> Heterostructure and Its Applications as a Supercapacitor Electrode and Photocatalyst for Reduction of Cr(VI) to Cr(III)

Ajay Lathe, Aleem Ansari, Rashmi A. Badhe, Anil M. Palve, Shivram S. Garje

2021ACS Omega55 citationsDOIOpen Access PDF

Abstract

In this study, we have reported a one-step synthesis of a TiO2@MoS2 heterostructure. TiO2@MoS2 was synthesized using a facile and cost-effective method. The as-synthesized TiO2@MoS2 heterostructure was characterized by suitable spectroscopic techniques. The obtained TiO2@MoS2 was utilized as a supercapacitor electrode material. Electrochemical studies show that the TiO2@MoS2 heterostructure possesses a specific capacitance of 337 F/g at a current density of 1 A/g in an aqueous solution. Furthermore, an application as a photocatalyst for the photoreduction of toxic hexavalent chromium was reported for the first time. This heterostructure showed the photoreduction of Cr6+ to Cr3+ in 120 min with formic acid as a scavenger under direct sunlight. A plausible mechanism of photoreduction of Cr6+ to Cr3+ under natural sunlight irradiation using TiO2@MoS2 is proposed.

Topics & Concepts

HeterojunctionPhotocatalysisMaterials scienceFormic acidHexavalent chromiumSupercapacitorElectrochemistryElectrodeAqueous solutionCapacitanceChromiumDegradation (telecommunications)IrradiationChemical engineeringOptoelectronicsCatalysisChemistryMetallurgyElectronic engineeringPhysical chemistryChromatographyNuclear physicsBiochemistryEngineeringPhysicsAdvanced Photocatalysis TechniquesAdvanced Nanomaterials in CatalysisSupercapacitor Materials and Fabrication