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(3,5-dimethyl-1H-pyrazol-1-y1) (4-((3,4-dimethoxybenzylidene) amino) phenyl) methanone as a novel corrosion inhibitor for low-carbon steel in hydrochloric acid: Synthesis, diagnosis, and application

Ali Shareef Jasim, Anees A. Khadom, Khalid H. Rashid, Khalida F. Al‐Azawi

2022Results in Chemistry26 citationsDOIOpen Access PDF

Abstract

A novel organic corrosion inhibitor, named (3,5-dimethyl-1H-pyrazol-1-y1) (4-((3,4-dimethoxybenzylidene) amino) phenyl) methanone (DPMM) has been effectively synthesized and characterized. FTIR has been used to diagnose DPMM's functional groups and components. Electrochemical and weight loss methods were used to assess the inhibitor efficacy for low-carbon steel in 1 M HCl. By raising the temperature and DPMM concentrations, the inhibition efficiency improved. The inhibition efficiency peaks at 95.5 % at 400 ppm of DPMM and 60 oC. The efficiency of the inhibitor was ascribed to the formation of a protective mono-layer on the steel surface. The mechanism of the adsorption process was examined using the Langmuir adsorption isotherm, whereas the mechanism of inhibition was examined using theoretical quantum chemical simulations. The results revealed that the DPMM was the donor of electron, while the steel surface was an electron acceptor.

Topics & Concepts

Hydrochloric acidAdsorptionLangmuir adsorption modelCarbon steelCorrosionNuclear chemistryChemistryElectrochemistryFourier transform infrared spectroscopyAcceptorMaterials scienceInorganic chemistryOrganic chemistryPhysical chemistryChemical engineeringElectrodeEngineeringPhysicsCondensed matter physicsCorrosion Behavior and InhibitionConcrete Corrosion and DurabilityHydrogen embrittlement and corrosion behaviors in metals
(3,5-dimethyl-1H-pyrazol-1-y1) (4-((3,4-dimethoxybenzylidene) amino) phenyl) methanone as a novel corrosion inhibitor for low-carbon steel in hydrochloric acid: Synthesis, diagnosis, and application | Litcius