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Synthesis and Characterization of Cellulose Triacetate Obtained from Date Palm (Phoenix dactylifera L.) Trunk Mesh-Derived Cellulose

Hamid Shaikh, Arfat Anis, Anesh Manjaly Poulose, Saeed M. Al‐Zahrani, Niyaz Ahamad Madhar, Abdullah Alhamidi, Saleh Husam Aldeligan, Faisal S. Alsubaie

2022Molecules63 citationsDOIOpen Access PDF

Abstract

Cellulosic polysaccharides have increasingly been recognized as a viable substitute for the depleting petro-based feedstock due to numerous modification options for obtaining a plethora of bio-based materials. In this study, cellulose triacetate was synthesized from pure cellulose obtained from the waste lignocellulosic part of date palm (Phoenix dactylifera L.). To achieve a degree of substitution (DS) of the hydroxyl group of 2.9, a heterogeneous acetylation reaction was carried out with acetic anhydride as an acetyl donor. The obtained cellulose ester was compared with a commercially available derivative and characterized using various analytical methods. This cellulose triacetate contains approximately 43.9% acetyl and has a molecular weight of 205,102 g·mol−1. The maximum thermal decomposition temperature of acetate was found to be 380 °C, similar to that of a reference sample. Thus, the synthesized ester derivate can be suitable for fabricating biodegradable and “all cellulose” biocomposite systems.

Topics & Concepts

Cellulose triacetateCelluloseAcetic anhydrideCellulose acetatePhoenix dactyliferaRaw materialOrganic chemistryChemistryMaterials sciencePolymer chemistryNuclear chemistryPalmPhysicsQuantum mechanicsCatalysisAdvanced Cellulose Research StudiesNatural Fiber Reinforced Compositesbiodegradable polymer synthesis and properties
Synthesis and Characterization of Cellulose Triacetate Obtained from Date Palm (Phoenix dactylifera L.) Trunk Mesh-Derived Cellulose | Litcius