Litcius/Paper detail

An Iridium/Aluminum Cooperative Strategy for the β‐C(sp<sup>3</sup>)‐H Borylation of Saturated Cyclic Amines

Yusuke Kuroda, Kyungho Park, Yuto Shimazaki, Rong‐Lin Zhong, Shigeyoshi Sakaki, Yoshiaki Nakao

2023Angewandte Chemie International Edition28 citationsDOI

Abstract

Abstract Despite the widespread success in the functionalization of C(sp 2 )−H bonds, the deliberate functionalization of C(sp 3 )−H bonds in a highly site‐ and stereoselective manner remains a longstanding challenge. Herein, we report an iridium/aluminum cooperative catalytic system that enables the β‐selective C−H borylation of saturated cyclic amines and lactams. Furthermore, we have accomplished an enantioselective variant using binaphthol‐derived chiral aluminum catalysts to forge C−B bonds with high levels of stereocontrol. Computational studies suggest that the formation of a Lewis pair with the substrates is crucial to lower the energy of the transition state for the rate‐determining reductive elimination step.

Topics & Concepts

BorylationIridiumEnantioselective synthesisCatalysisChemistryStereoselectivityCombinatorial chemistryAluminiumSurface modificationMedicinal chemistryStereochemistryOrganic chemistryPhysical chemistryAlkylArylCatalytic C–H Functionalization MethodsOrganoboron and organosilicon chemistryAsymmetric Hydrogenation and Catalysis