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Organocatalytic atroposelective synthesis of axially chiral <i>N</i>,<i>N</i>′-pyrrolylindoles <i>via de novo</i> indole formation

Cong-Shuai Wang, Qi Xiong, Hui Xu, Haoran Yang, Yanfeng Dang, Xiu‐Qin Dong, Chun‐Jiang Wang

2023Chemical Science33 citationsDOIOpen Access PDF

Abstract

The first organocatalytic atroposelective synthesis of chiral N,N ′-pyrrolylindoles based on CPA-catalyzed asymmetric 5- endo-dig cyclization of well-designed o -alkynylanilines bearing pyrrolyl unit was established via de novo indole formation.

Topics & Concepts

Indole testChemistryAxial symmetryStereochemistryCombinatorial chemistryPhysicsQuantum mechanicsAxial and Atropisomeric Chirality SynthesisMolecular spectroscopy and chirality