Litcius/Paper detail

Synergistic and Antagonistic Effects of the Co-Pyrolysis of Plastics and Corn Stover to Produce Char and Activated Carbon

Mark Gale, Peter M. Nguyen, Kandis Leslie Gilliard‐AbdulAziz

2022ACS Omega20 citationsDOIOpen Access PDF

Abstract

/g at 500 °C and a duration of 2 h. The surface area of the chars formed from CS and PET decreased as the amount of PET decreased, showing a tendency for PET to increase the surface area of the char materials synergistically. The addition of PS to corn stover promoted the formation of chars with, on average, larger pore sizes than the control char samples. The chars were chemically activated with potassium hydroxide, and the activated carbon that formed had lower surface areas but comparable surface functional groups to the control samples. Vanillin adsorption testing showed that activated carbon from corn stover performed the best at removing 95% of the vanillin after 2 h. In contrast, the activated carbon from the chars produced from the co-pyrolysis of corn stover and polystyrene or corn stover and polyethylene terephthalate removed 45% and 46% of vanillin after 2 h, respectively. The findings suggest that plastics have a synergistic relationship in producing char precursors with improved porosity but antagonistically affect the activated carbon adsorbent properties.

Topics & Concepts

CharCorn stoverActivated carbonPotassium hydroxidePyrolysisAdsorptionChemistrySpecific surface areaPolyethylene terephthalateChemical engineeringPolystyreneCarbon fibersVanillinNuclear chemistryMaterials scienceOrganic chemistryComposite materialPolymerFermentationComposite numberCatalysisEngineeringMicroplastics and Plastic PollutionRecycling and Waste Management TechniquesThermochemical Biomass Conversion Processes