Litcius/Paper detail

Hydrogen Bonds Defined Pore Windows Enable Sieving Separation of Propylene from Propane in an Ultramicroporous Metal–Organic Framework

Xiang‐Jing Kong, Mingming Xu, Tao He, Lin‐Hua Xie, Yuhui Liu, Xin Zhang, Hao-Tian Wang, Jian‐Rong Li

2024Chemistry of Materials8 citationsDOI

Abstract

Tailoring a MOF with suitable pore windows for the sieving C 3 H 6 /C 3 H 8 separation is attractive but challenging, where controlling the local framework flexibility by introducing functionality provides a solution. In this work, four isoreticular ultramicroporous Zn–triazolate–dicarboxylate frameworks, Zn-ATZ-IP(R) (R = −F, −OH, −NH 2, and −CH 3 ) (HATZ = 3-amino-1,2,4-triazole; H 2 IP-R = R group functionalized isophthalic acid) with variable pore apertures, were targeted as platforms to study the effect of functional groups on their separation performance. Single-component adsorption isotherms uncovered the potential of Zn-ATZ-IP(OH)-a with hydroxyl groups as a sieving adsorbent. Single X-ray diffraction (SXRD) measurements revealed that strong intraframework hydrogen bonds hinder the free torsion of ATZ – ligand in Zn-ATZ-IP(OH)-a, defining rigid pore windows that admit C 3 H 6 while exclude C 3 H 8, whereas other groups give adaptive larger pores that allow both C 3 H 6 and C 3 H 8 in. Further, in situ XRD measurements suggested that temperature alters the strength of hydrogen bonds, making Zn-ATZ-IP(OH)-a ideal for room-temperature sieving of C 3 H 6 /C 3 H 8 . This work highlights the superiority of customizing sieving pores sustained by hydrogen bonds, which advances the rational design of smart adsorbents for energy-efficient light hydrocarbon separations.

Topics & Concepts

PropaneMetal-organic frameworkHydrogen bondMaterials scienceChemical engineeringMetalPropeneOrganic chemistryChemistryAdsorptionCatalysisMoleculeEngineeringMetal-Organic Frameworks: Synthesis and ApplicationsMesoporous Materials and CatalysisCovalent Organic Framework Applications